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Experimental and theoretical study of microwave enhanced catalytic hydrodesulfurization of thiophene

Hui Shang, Pengfei Ye, Yude Yue, Tianye Wang, Wenhui Zhang, Sainab Omar, Jiawei Wang

《化学科学与工程前沿（英文）》 2019年 第13卷 第4期   页码 744-758 doi: 10.1007/s11705-019-1839-7

摘要： Hydrodesulfurization (HDS) of thiophene, as a gasoline model oil, over an industrial Ni-Mo/Al O catalyst was investigated in a continuous system under microwave irradiation. The HDS efficiency was much higher (5%‒14%) under microwave irradiation than conventional heating. It was proved that the reaction was enhanced by both microwave thermal and non-thermal effects. Microwave selective heating caused hot spots inside the catalyst, thus improved the reaction rate. From the analysis of the non-thermal effect, the molecular collisions were significantly increased under microwave irradiation. However, instead of being reduced, the apparent activation energy increased. This may be due to the microwave treatment hindering the adsorption though upright S-bind (η ) and enhancing the parallel adsorption (η ), both adsorptions were considered to favor to the direct desulfurization route and the hydrogenation route respectively. Therefore, the HDS process was considered to proceed along the hydrogenation route under microwave irradiation.

关键词： thiophene     microwave irradiation     hydrodesulfurization     non-thermal microwave effect    

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NOx removal by non-thermal plasma reduction: experimental and theoretical investigations

《化学科学与工程前沿（英文）》 2022年 第16卷 第10期   页码 1476-1484 doi: 10.1007/s11705-022-2165-z

摘要： Green and efficient NOx removal at low temperature is still desired. NOx removal via non-thermal plasma (NTP) reduction is one of such technique. This work presents the experimental and theoretical study on the NOx removal via NTP reduction (NTPRD) in dielectric barrier discharge reactor (DBD). The effect of O2 molar fraction on NOx species in the outlet of DBD, and effects of NH3/NO molar ratio and discharge power of DBD on NOx removal efficiency are investigated. Results indicate that anaerobic condition and higher discharge power is beneficial to direct removal of NOx, and the NOx removal efficiency can be up to 98.5% under the optimal operating conditions. It is also found that adding NH3 is favorable for the reduction of NOx to N2 at lower discharge power. In addition, the NOx removal mechanism and energy consumption analysis for the NTPRD process are also studied. It is found that the reduced active species ( N∗, N−, N+, N2∗, NH2+, etc.) generated in the NTPRD process play important roles for the reduction of NOx to N2. Our work paves a novel pathway for NOx removal from anaerobic gas in industrial application.

关键词： ${\rm{NO}}_x $ removal     NTP reduction     mechanism     energy consumption    

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Non-thermal plasma enhances performances of biochar in wastewater treatment and energy storage applications

《化学科学与工程前沿（英文）》 2022年 第16卷 第4期   页码 475-483 doi: 10.1007/s11705-021-2070-x

摘要： Surface functionalization or modification to introduce more oxygen-containing functional groups to biochar is an effective strategy for tuning the physicochemical properties and promoting follow-up applications. In this study, non-thermal plasma was applied for biochar surface carving before being used in contaminant removal and energy storage applications. The results showed that even a low dose of plasma exposure could introduce a high number density of oxygen-functional groups and enhance the hydrophilicity and metal affinity of the pristine biochar. The plasma-treated biochar enabled a faster metal-adsorption rate and a 40% higher maximum adsorption capacity of heavy metal ion Pb2+. Moreover, to add more functionality to biochar surface, biochar with and without plasma pre-treatment was activated by KOH at a temperature of 800 °C. Using the same amount of KOH, the plasma treatment resulted in an activated carbon product with the larger BET surface area and pore volume. The performance of the treated activated carbon as a supercapacitor electrode was also substantially improved by>30%. This study may provide guidelines for enhancing the surface functionality and application performances of biochar using non-thermal-based techniques.

关键词： non-thermal plasma     surface functionalization     biochar modification     wastewater treatment     supercapacitor    

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Plasma-catalysis: Is it just a question of scale?

J. Christopher Whitehead

《化学科学与工程前沿（英文）》 2019年 第13卷 第2期   页码 264-273 doi: 10.1007/s11705-019-1794-3

摘要： The issues of describing and understanding the changes in performance that result when a catalyst is placed into plasma are discussed. The different chemical and physical interactions that result and how their combination might produce beneficial results for the plasma-catalytic processing of different gas streams are outlined with particular emphasis being placed on the different range of spatial and temporal scales that must be considered both in experiment and modelling. The focus is on non-thermal plasma where the lack of thermal equilibrium creates a range of temperature scales that must be considered. This contributes in part to a wide range of inhomogeneity in different properties such as species concentrations and electric fields that must be determined experimentally by methods and be incorporated into modelling. It is concluded that plasma-catalysis is best regarded as conventional catalysis perturbed by the presence of a discharge, which modifies its operating conditions, properties and outcomes often in a very localised way. The sometimes used description “plasma-activated catalysis” is an apt one.

关键词： plasma catalysis     plasma-activated catalysis     non-thermal plasma     CO2 conversion    

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Benzene conversion by manganese dioxide assisted silent discharge plasma

LU Bin, JI Min, YU Xin, FENG Tao, YAO Shuiliang

《环境科学与工程前沿（英文）》 2007年 第1卷 第4期   页码 477-481 doi: 10.1007/s11783-007-0076-3

摘要： Non-thermal plasma technologies have shown their promising potential specially for the low concentration of volatile organic compound control in indoor air in recent years. But it is also high energy consuming. So, to improve the en

关键词： consuming     Non-thermal     promising     volatile     compound    

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Assessment indices for uniform and non-uniform thermal environments

ZHANG Yufeng, SUN Shufeng, ZHAO Rongyi

《能源前沿（英文）》 2008年 第2卷 第2期   页码 129-133 doi: 10.1007/s11708-008-0029-y

摘要： Different assessment indices for thermal environments were compared and selected for proper assessment of indoor thermal environments. 30 subjects reported their overall thermal sensation, thermal comfort, and thermal acceptability in uniform and non-uniform conditions. The results show that these three assessment indices provide equivalent evaluations in uniform environments. However, overall thermal sensation differs from the other two indices and cannot be used as a proper index for the evaluation of non-uniform environments. The relationship between the percentage and the mean vote for each index is established.

关键词： thermal sensation     proper assessment     relationship     equivalent     thermal acceptability    

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Non-thermal plasma for exhaust gases treatment

Elvia ALVA R.,Marquidia PACHECO P.,Fernando GÓMEZ B.,Joel PACHECO P.,Arturo COLÍN C.,Víctor SÁNCHEZ-MENDIETA,Ricardo VALDIVIA B.,Alfredo SANTANA D.,José HUERTAS C.,Hilda FRÍAS P.

《机械工程前沿（英文）》 2015年 第10卷 第3期   页码 301-305 doi: 10.1007/s11465-015-0344-z

摘要：

This article describes a study on a non-thermal plasma device to treat exhaust gases in an internal combustion engine. Several tests using a plasma device to treat exhaust gases are conducted on a Honda GX200-196 cm3 engine at different rotational speeds. A plasma reactor could be efficient in degrading nitrogen oxides and particulate matter. Monoxide and carbon dioxide treatment is minimal. However, achieving 1%–3% degradation may be interesting to reduce the emission of greenhouse gases.

关键词： plasma treatment     NOx     CO     CO2     particulate matter     vehicle    

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Thermal analysis of lubricated three-dimensional contact bodies considering interface roughness

《机械工程前沿（英文）》 2022年 第17卷 第2期 doi: 10.1007/s11465-022-0672-8

摘要： Surface roughness and thermal action are of remarkable importance in the lubrication performance of mechanical components, especially in extreme conditions. However, available studies mainly focus on the full-film lubrication conditions without considering temperature rise and real 3D surface roughness due to the complexity of surface topography and temperature characteristics. Moreover, studies on the interfacial thermal behaviors of 3D rough surface lubricated contact in an extended range of working conditions remain limited. In this paper, a deterministic mixed thermal elastohydrodynamic lubrication model considering real 3D surface roughness and thermal effects is proposed. In this model, pressure and temperature are coupled with each other, the computation of elastic deformation is accelerated through the discrete convolution and fast Fourier transform method, the temperature field is calculated with the column sweeping technique, and the semi-system method is introduced to improve convergence and numerical stability under severe conditions. The model is validated by comparing its results with available published numerical and experimental results. The thermal behaviors of the contact interface are studied in a wide range of working conditions. The influences of surface roughness and thermal effect on lubrication performance are revealed. The results show that the proposed model can be used as a powerful analysis tool for lubrication performance and temperature prediction in various heavy-load, high-speed lubricated components over a wide range of lubrication conditions.

关键词： thermal elastohydrodynamic lubrication     surface roughness effect     thermal effect     temperature characteristics     severe conditions    

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FY-3B卫星微波湿度计热真空定标方法和结果分析

王振占,张升伟,李靖,李芸,吴琼

《中国工程科学》 2013年 第15卷 第10期   页码 33-46

摘要：

本文论述了风云三号卫星B星微波湿度计（MWHS-3B）发射前热真空定标的原理和方法，建立了各种定标误差的修正算法，获得了MWHS-3B的系统线性度、观测不同目标的灵敏度和最终定标精度等关键技术指标。这些参数已经用于MWHS-3B在轨数据的处理。

关键词： 风云三号卫星     微波湿度计     发射前定标     热真空定标    

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Greenhouse gas emissions from thermal treatment of non-recyclable municipal waste

Tomáš Ferdan, Martin Pavlas, Vlastimír Nevrlý, Radovan Šomplák, Petr Stehlík

《化学科学与工程前沿（英文）》 2018年 第12卷 第4期   页码 815-831 doi: 10.1007/s11705-018-1761-4

摘要：

This paper analyses factors affecting the production of greenhouse gases from the treatment of residual municipal waste. The analysis is conducted so that the environmentally-friendly decision-making criteria may be later implemented into an optimisation task, which allocates waste treatment capacities. A simplified method of life cycle assessment is applied to describe environmental impact of the allocation. Global warming potential (GWP) is employed as a unit to quantify greenhouse gases (GHG) emissions. The objective is to identify the environmental burdens and credits measured by GWP for the three fundamental methods for treatment of residual waste unsuitable for material recovery. The three methods are waste-to-energy (WTE), landfilling and mechanical-biological treatment (MBT) with subsequent utilization of refuse-derived fuel. The composition of the waste itself and content of fossil-derived carbon and biogenic carbon are important parameters to identify amounts of GHG. In case of WTE, subsequent use of the energy, e.g., in district heating systems in case of heat, is another important parameter to be considered. GWP function dependant on WTE capacity is introduced. The conclusion of this paper provides an assessment of the potential benefits of the results in optimisation tasks for the planning of overall strategy in waste management.

关键词： waste management     greenhouse gases     global warming potential     allocation planning     waste-to-energy    

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Effect of thermal pretreatment on the surface structure of PtSn/SiO

Guozhen Xu, Jian Zhang, Shengping Wang, Yujun Zhao, Xinbin Ma

《化学科学与工程前沿（英文）》 2016年 第10卷 第3期   页码 417-424 doi: 10.1007/s11705-016-1583-1

摘要： The effect of thermal pretreatment on the active sites and catalytic performances of PtSn/SiO catalyst in acetic acid (AcOH) hydrogenation was investigated in this article. The catalysts were characterized by N physical adsorption, X-ray diffraction, transmission electron microscopy, pyridine Fourier-transform infrared spectra, and H -O titration on its physicochemical properties. The results showed that Pt species were formed primarily in crystalline structure and no PtSn alloy was observed. Meanwhile, with the increment of thermal pretreatment temperature, Pt dispersion showed a decreasing trend due to the aggregation of Pt particles. Simultaneously, the amount of Lewis acid sites was remarkably influenced by such thermal pretreatment owning to the consequent physicochemical property variation of Sn species. Interestingly, the catalytic activity showed the similar variation trend with that of Lewis acid sites, confirming the important roles of Lewis acid sites in AcOH hydrogenation. Moreover, a balancing effect between exposed Pt and Lewis acid sites was obtained, resulting in the superior catalytic performance in AcOH hydrogenation.

关键词： thermal pretreatment     acetic acid     hydrogenation     ethanol     PtSn/SiO2    

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Effect of non-uniform illumination on performance of solar thermoelectric generators

Ershuai YIN, Qiang LI, Yimin XUAN

《能源前沿（英文）》 2018年 第12卷 第2期   页码 239-248 doi: 10.1007/s11708-018-0533-7

摘要： Solar thermoelectric generators (STEGs) are heat engines which can generate electricity from concentrated sunlight. The non-uniform illumination caused by the optical concentrator may affect the performance of solar thermoelectric generators. In this paper, a three-dimensional finite element model of solar thermoelectric generators is established. The two-dimensional Gaussian distribution is employed to modify the illumination profiles incident on the thermoelectric generator. Six non-uniformities of solar illumination are investigated while keeping the total energy constant. The influences of non-uniform illumination on the temperature distribution, the voltage distribution, and the maximum output power are respectively discussed. Three thermoelectric generators with 32, 18 and 8 pairs of thermocouples are compared to investigate their capability under non-uniform solar radiation. The result shows that the non-uniformity of the solar illumination has a great effect on the temperature distribution and the voltage distribution. Central thermoelectric legs can achieve a larger temperature difference and generate a larger voltage than peripheral ones. The non-uniform solar illumination will weaken the capability of the TE generator, and the maximum output power decrease by 1.4% among the range of non-uniformity studied in this paper. Reducing the number of the thermoelectric legs for non-uniform solar illumination can greatly increase the performance of the thermoelectric generator.

关键词： solar thermoelectric generators     non-uniform solar illumination     performance evaluation     solar energy    

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非爆炸且不可还原农用硝酸铵的热稳定性评估

汪旭光,沈立晋

《中国工程科学》 2004年 第6卷 第11期   页码 53-57

摘要：

绍了一种测试含能材料热稳定性的新方法——加速度量热仪，并用此法研究了硝酸铵和非爆炸且不可还原农用硝酸铵的热分解过程，得到了绝热分解温度与压力随时间的变化、自加热速率与分解压力随温度的变化曲线，计算了分解动力学参数表观活化能和指前因子，讨论了放热反应系统的热惰性因子对测试结果的影响，表明非爆炸且不可还原农用硝酸铵具有良好的热稳定性、安全性及其热稳定性的提高是爆炸特性得以消除的原因。

关键词： 农用硝酸铵     非爆炸性     不可还原性     加速度量热仪     热稳定性    

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CD47 blockade improves the therapeutic effect of osimertinib in non-small cell lung cancer

《医学前沿（英文）》 2023年 第17卷 第1期   页码 105-118 doi: 10.1007/s11684-022-0934-1

摘要： The third-generation epidermal growth factor receptor (EGFR) inhibitor osimertinib (OSI) has been approved as the first-line treatment for EGFR-mutant non-small cell lung cancer (NSCLC). This study aims to explore a rational combination strategy for enhancing the OSI efficacy. In this study, OSI induced higher CD47 expression, an important anti-phagocytic immune checkpoint, via the NF-κB pathway in EGFR-mutant NSCLC HCC827 and NCI-H1975 cells. The combination treatment of OSI and the anti-CD47 antibody exhibited dramatically increasing phagocytosis in HCC827 and NCI-H1975 cells, which highly relied on the antibody-dependent cellular phagocytosis effect. Consistently, the enhanced phagocytosis index from combination treatment was reversed in CD47 knockout HCC827 cells. Meanwhile, combining the anti-CD47 antibody significantly augmented the anticancer effect of OSI in HCC827 xenograft mice model. Notably, OSI induced the surface exposure of “eat me” signal calreticulin and reduced the expression of immune-inhibitory receptor PD-L1 in cancer cells, which might contribute to the increased phagocytosis on cancer cells pretreated with OSI. In summary, these findings suggest the multidimensional regulation by OSI and encourage the further exploration of combining anti-CD47 antibody with OSI as a new strategy to enhance the anticancer efficacy in EGFR-mutant NSCLC with CD47 activation induced by OSI.

关键词： osimertinib     anti-CD47 antibody     combination strategy     ADCP     EGFR    

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标题 作者 时间 类型 操作

Experimental and theoretical study of microwave enhanced catalytic hydrodesulfurization of thiophene

Hui Shang, Pengfei Ye, Yude Yue, Tianye Wang, Wenhui Zhang, Sainab Omar, Jiawei Wang

期刊论文

NOx removal by non-thermal plasma reduction: experimental and theoretical investigations

期刊论文

Non-thermal plasma enhances performances of biochar in wastewater treatment and energy storage applications

期刊论文

Plasma-catalysis: Is it just a question of scale?

J. Christopher Whitehead

期刊论文

Benzene conversion by manganese dioxide assisted silent discharge plasma

LU Bin, JI Min, YU Xin, FENG Tao, YAO Shuiliang

期刊论文

宋华：廉价碳源非热等离子光催化改制技术研究（2022年4月16日）

2022年06月09日

会议视频

Assessment indices for uniform and non-uniform thermal environments

ZHANG Yufeng, SUN Shufeng, ZHAO Rongyi

期刊论文

Non-thermal plasma for exhaust gases treatment

Elvia ALVA R.,Marquidia PACHECO P.,Fernando GÓMEZ B.,Joel PACHECO P.,Arturo COLÍN C.,Víctor SÁNCHEZ-MENDIETA,Ricardo VALDIVIA B.,Alfredo SANTANA D.,José HUERTAS C.,Hilda FRÍAS P.

期刊论文

Thermal analysis of lubricated three-dimensional contact bodies considering interface roughness

期刊论文

FY-3B卫星微波湿度计热真空定标方法和结果分析

王振占,张升伟,李靖,李芸,吴琼

期刊论文

Greenhouse gas emissions from thermal treatment of non-recyclable municipal waste

Tomáš Ferdan, Martin Pavlas, Vlastimír Nevrlý, Radovan Šomplák, Petr Stehlík

期刊论文

Effect of thermal pretreatment on the surface structure of PtSn/SiO

Guozhen Xu, Jian Zhang, Shengping Wang, Yujun Zhao, Xinbin Ma

期刊论文

Effect of non-uniform illumination on performance of solar thermoelectric generators

Ershuai YIN, Qiang LI, Yimin XUAN

期刊论文

非爆炸且不可还原农用硝酸铵的热稳定性评估

汪旭光,沈立晋

期刊论文

CD47 blockade improves the therapeutic effect of osimertinib in non-small cell lung cancer

期刊论文